理论和物理化学

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节家龙                


                     

副教授,博士生导师,理学学士(上海交通大学),理学博士(中国科学院化学研究所),博士后(美国俄亥俄州立大学)



通信地址:北京市新街口外大街19号,北京师范大学化学学院K102


邮编:100875                


电子邮箱:jialong@bnu.edu.cn                


课题组主页:http://chem1.bnu.edu.cn/shm/              

             


讲授课程

物理化学B/ C(化学动力学基础和分子反应动力学章节)、化学基础实验II


研究兴趣

自由基和激发态是高反应活性的瞬态物种,是影响多种化学、生物过程的关键活泼中间体。我们致力于发展和运用多种时间分辨激光光谱技术,以能源、环境、材料和生命科学中的一些基础科学问题为背景,探测一系列重要的自由基及激发态分子的反应动力学过程,结合量子化学计算,深入阐述反应微观机理。研究方向主要包括生物分子DNA/蛋白质光响应、光催化有机合成反应等凝聚相体系中各种复杂的物理化学动态过程,涉及化学动力学、分子光化学、分子光生物、激光光谱等领域中的前沿基础。


承担科研项目

1. 可见光氧化还原催化脱羧偶联反应的微观机制及动力学研究,国家自然科学基金面上项目(2247301450万),2025.01-2028.12,主持

2. UV光诱导S-DNA氧化损伤反应动力学机制的研究,国家自然科学基金青年科学基金项目(2200300530万)2021.01-2023.12,主持,结题

3. 紫外光诱导硫代核酸氧化损伤反应动力学机制的研究,北京师范大学青年教师基金项目(2020NTST1010万)2020.10-2022.09,主持,结题

4. 磁场调控光氧化还原催化有机合成,国家重点研发计划青年科学家项目(2022YFA1505400500万),2022.12-2027.11,项目骨干

5. 优秀青年创新团队项目(2233300007400万),2023.09-2025.09,项目骨干

6. 修饰碱基及其在不同DNA结构中的单电子氧化和脱质子反应机理研究,国家自然科学基金面上项目(2227300754万),2023.01-2026.12,项目骨干

代表性论文

21. Mingli Sun, Jie Cheng, Chenli Chen, Jialong Jie*, Hongmei Su, Song Gao, and Linan Zhou*, Viscosity-Controlled Magnetic Field Effects in Homogeneous Photoredox Catalysis Enabled by Ionic Liquids, Molecules, 2026, 31, 886.

20. Mingming Yu*, Jing Feng, Xingyu Wang, Xinyuan Xiang, Ye Hu, Ze-Hua Wang, Ze-Feng Xu, Jialong Jie*, Hongmei Su*, Hao Tang*, and Chuan-Ying Li*, Photo-induced selective N-N bond construction via harnessing nitrene release and transfer, Nat. Commun. 2026, 17, 2084.

19. Mingli Sun, Chenli Chen, Lingfang Chen, Jiayi Liang, Jie Cheng, Jialu Li, Shuming Bai*, Jialong Jie*, Hongmei Su, Song Gao, and Linan Zhou*, Synergistic Enhancement of Photoredox Catalysis Beyond the Singlet Bottleneck Through Triplet Charge Recombination and Magnetic Field Effects, Angew. Chem. Int. Ed. 2026, 65, e18648.

18. Xiaogang Tong#, Jialong Jie#, Yan Liu, Haihan Yu, Mingquan Yuan, Hwee Ting Ang, GanWang, Duanshuai Tian, Hongmei Su*, and Jie Wu*, Photocatalytic streamlined dual-functional group transfer from cyanopyridine to internal alkynes, Nat. Commun. 2025, 16, 8985.

17. Siwei Wu#, Jialong Jie#, Lin Liu#, Linshan Liu#, Shengzhu Guo, Xiaonan Li, Jing He, Zhe Lian, Ying Wang,* Xinjun Xu,* Hongmei Su,* Xuebo Chen,* and Hua Jiang*, A Redox-Active π-Extended Tetrathiafulvalene-Based Carbon Nanohoop Featuring Unique Kasha/Anti-Kasha Dual Emissions: Structure, Photophysical Properties, and Photoconductivity, Angew. Chem. Int. Ed. 2025, 64, e202512167.

16. Zhiqiang Dong, Chenli Chen, Lingfang Chen, Mingli Sun, Junzheng Zhan, Shen Zhou, Lijia Cao, Jianyu Liu, Shuming Bai*, Jialong Jie*, Hongmei Su, Song Gao, and Linan Zhou*, Enhancing photoredox catalysis by suppressing back electron transfer with the aid of a spin catalyst, Chem. Sci. 2025, 16, 17276-17286.

15. Jing-dong Zhang#, Jia-long Jie#,*, Shu-yi Yan, Hui Zhang, Jia-meng Chen, Jiang-cheng Wu, Lu-yang Qin, Guang-jian Liu, Hong-mei Su, and Guo-wen Xing*, Single electron/energy transfer photocatalysis: α-/β-switchable synthesis of 3-deoxy-D-manno-oct-2-ulosonic acid O-glycosides, Chem. Sci. 2025, 16, 13070-13081.

14. Zeqing Jiao, Chen Wang, Qian Zhou, Jialong Jie*, and Hongmei Su*, Enhanced Triplet State of Coralyne via DNA-Templated Gold Nanostars, Chin. J. Chem. Phys. 2025, 38, 711-720.

13. Shuyi Yan#, Wenwen Guo#, Jialong Jie#, Qian Zhou, Di Song*, Dongyu Li, and Hongmei Su*, Protonation Weakens the Influence of Ribose on Triplet Decay of 2-Thiocytidine, J. Phys. Chem. Lett. 2024, 15, 47, 11839-11846.

12. Zhicong Lin#, Jialu Li#, Chenli Chen, Linan Zhou*, Jialong Jie*, and Hongmei Su*, Mechanistic Study of Initial Quenching Process in Photocatalytic α-Keto Acids Radical Acylation: A General Strategy for Enhancing Quantum Efficiency, Chin. J. Chem. Phys. 2024, 37, 878-892.

11. Qian Zhou#, Wenwen Guo#, Zheng Hu, Shuyi Yan, Jialong Jie*, and Hongmei Su*, Can methylated purine bases act as photoionization hotspots?, Photochem. Photobio. 2024, 100, 368-379.

10. Zhicong Lin#, Qian Zhou#, Yan Liu, Chenli Chen, Jialong Jie*, and Hongmei Su, Multiphoton tandem photoredox catalysis of [Ir(dFCF3ppy)2(dtbbpy)]+ facilitating radical acylation reactions, Chem. Sci. 2024, 15, 11919-11927.

9. Chunfan Yang, Fang Wang, Qian Zhou, Jialong Jie*, and Hongmei Su*, Fluorescence Quenching Dynamics of 2-Amino-7-methyl-1,8-naphthyridine in Abasic-Site-Containing DNA Duplexes for Nucleobase Recognition, J. Phys. Chem. Lett. 2023, 14, 10585-10591.

8. Zeqing Jiao, Chunfan Yang, Qian Zhou, Zheng Hu, Jialong Jie*, Xianwang Zhang, and Hongmei Su*, Sequence-specific binding behavior of coralyne toward triplex DNA: An ultrafast time-resolved fluorescence spectroscopy study, J. Chem. Phys. 2023, 158, 045101.

7. Zheng Hu, Qian Zhou, Zeqing Jiao, Peixuan Qin, Fei Wang, Ye Xia, Tianfeng Zhang, Jialong Jie*, and Hongmei Su*, Low Energy Photoionization of Phosphorothioate DNA-Oligomers and Ensuing Hole Transfer, J. Phys. Chem. B 2022, 126, 8699-8707.

6. Junjie Dong#, Chunhua Huang#, Shaoshi Guo#, Ye Xia, Yue Hou, Chunfan Yang, Xianwang Zhang, Jialong Jie*, Ben-zhan Zhu, and Hongmei Su*, Free-Radical-Mediated Photoinduced Electron Transfer between 6-Thioguanine and Tryptophan Leading to DNA-Protein-Like Cross-Link, J. Phys. Chem. B 2022, 126, 14-22.

5. Haihui Peng#, Jialong Jie#, Ifor P. Mortimer, Zehan Ma, Hongmei Su*, and Marc M. Greenberg*, Reactivity and DNA Damage by Independently Generated 2′-Deoxycytidin-N4-yl Radical, J. Am. Chem. Soc. 2021, 143, 14738-14747.

4. Xianwang Zhang, Jialong Jie*, Di Song*, and Hongmei Su, Deprotonation of Guanine Radical Cation G·+ Mediated by the Protonated Water Cluster, J. Phys. Chem. A 2020, 124, 6076-6083.

3. Jialong Jie, Ye Xia, Chunhua Huang, Hongmei Zhao, Chunfan Yang, Kunhui Liu, Di Song, BenZhan Zhu, and Hongmei Su*, Sulfur-centered Hemi-bond Radicals as Active Intermediates in S-DNA Phosphorothioate Oxidation, Nucleic Acids Res. 2019, 47, 11514-11526.

2. Jialong Jie, Kunhui Liu, Lidan Wu, Hongmei Zhao, Di Song, and Hongmei Su*, Capturing the Radical Ion-pair Intermediate in DNA Guanine Oxidation, Sci. Adv. 2017, 3, e1700171.

1. Jialong Jie, Chen Wang, Hongmei Zhao, Di Song*, and Hongmei Su*, Experimental and Theoretical Study of the Deprotonation of DNA Adenine Cation Radical, Chin. J. Chem. Phys. 2017, 30, 664-670.